Microporous waste charcoals for redox-mediated supercapacitors

Jong Chan Hyun; Jin Hwan Kwak; Young Soo Yun

Journal of Industrial and Engineering Chemistry, Vol.79, 204-209, November, 2019

DOI10.1016/j.jiec.2019.06.036 Export Citation

Microporous waste charcoals for redox-mediated supercapacitors

Jong Chan Hyun, Jin Hwan Kwak, and Young Soo Yun^†

Department of Chemical Engineering, Kangwon National University, Samcheok 245-711, South Korea

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The energy density of supercapacitors could be improved significantly using microporous carbon-based materials (MP-CMs) with multitudinous redox-active heteroatoms through the hybrid charge storage behaviors of both pseudocapacitance and electrochemical double layer capacitance in a redox-mediated aqueous electrolyte system. Waste-derived MP-CMs were prepared using a simple activation process and used as high-performance electrode materials for redox-mediated supercapacitors, showing a high specific capacitance of~512 F g-1 and a reasonable rate and cycling performance.

Keywords:Activated carbon;Porous carbon;Electrodes;Charcoal;Supercapacitor

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[1] Simon P, Gogotsi Y, Nat. Mater., 7, 845 (2008)

[2] Yun YS, Cho SY, Shim J, Kim BH, Chang SJ, Baek SJ, Huh YS, Tak Y, Park YW, Park S, Jin HJ, Adv. Mater., 25(14), 1993 (2013)

[3] Yun YS, Lee S, Kim NR, Kang M, Leal C, Park KY, Kang K, Jin HJ, J. Power Sources, 313, 142 (2016)

[4] Jiang H, Lee PS, Li C, Energy Environ. Sci., 6, 41 (2013)

[5] Xia K, Gao Q, Jiang J, Hu J, Carbon, 46, 1718 (2008)

[6] Yun YS, Park MH, Hong SJ, Lee ME, Park YW, Jin HJ, ACS Appl. Mater. Interfaces, 7, 3684 (2015)

[7] Zhao L, Fan LZ, Zhou MQ, Guan H, Qiao SY, Antonietti M, Titirici MM, Adv. Mater., 22(45), 5202 (2010)

[8] Hulicova-Jurcakova D, Seredych M, Lu GQ, Bandosz TJ, Adv. Funct. Mater., 19(3), 438 (2009)

[9] Ji H, Zhao X, Qiao Z, Jung J, Zhu Y, Lu Y, et al., Nat. Commun., 5, 3317 (2014)

[10] Biener J, Stadermann M, Suss M, Worsley MA, Biener MM, Rose KA, et al., Energy Environ. Sci., 4, 656 (2011)

[11] To JWF, Chen Z, Yao H, He JJ, Kim K, Chou HH, et al., ACS Cent. Sci., 1, 68 (2015)

[12] Zhang Y, Liu S, Zheng X, Wang X, Xu Y, Tang H, Kang F, Yang QH, Luo J, Adv. Funct. Mater., 27, 160468 (2017)

[13] Teo EYL, Muniandy L, Ng EP, Adam F, Mohamed AR, Jose R, Chong KF, Electrochim. Acta, 192, 110 (2016)

[14] Lee DY, Ah GH, Ahn HJ, J. Ind. Eng. Chem., 52, 121 (2017)

[15] Cho ES, Bai BC, Im JS, Lee CW, Kim S, J. Ind. Eng. Chem., 35, 341 (2016)

[16] Zhu YQ, Zhang L, Chen XY, Xiao ZH, Zhang ZJ, J. Power Sources, 299, 629 (2015)

[17] Zhang ZJ, Chen XY, J. Electroanal. Chem., 764, 45 (2016)

[18] Wu J, Yu H, Fan L, Luo G, Lin J, Huang M, J. Mater. Chem., 22, 19025 (2012)

[19] Roldan S, Blacno C, Granda M, Menendez R, Santamaria R, Angew. Chem.-Int. Edit., 50, 1699 (2011)

[20] Yu H, Fan L, Wu J, Lin Y, Huang M, Lin J, et al., RSC. Adv., 2, 6736 (2012)

[21] An HJ, Kim NR, Song MY, Yun YS, Jin HJ, J. Ind. Eng. Chem., 45, 223 (2017)

[22] Zhang ZJ, Zhu YQ, Chen XY, Cao Y, Electrochim. Acta, 176, 941 (2015)

[23] Yun YS, Yoon G, Kang K, Jin HJ, Carbon, 80, 246 (2014)

[24] Song MY, Kim NR, Cho SY, Jin HJ, Yun YS, ACS Sustainable Chem. Eng., 5, 616 (2017)