Recently, a new type of battery has been proposed that relies on the principle of self-assembling of a liquid metalloid positive electrode, a liquid electrolyte, and a liquid metal negative electrode. While this configuration has been claimed to allow arbitrary up-scaling, there is a size limitation of such a system due to a current-driven kink-type instability that is known as the Tayler instability. We characterize this instability in large-scale self-assembled liquid metal batteries and discuss various technical means how it can be avoided. (C) 2011 Elsevier Ltd. All rights reserved.