We report the formation of nanoclusters on the surface of gallium nitride (GaN) epilayers due to irradiation with 70 MeV Si ions with the fluences of 1 x 10(12) ions/cm(2) at the liquid nitrogen temperature (77 K). GaN epilayers were grown using a metal organic chemical vapor deposition system. Omega scan rocking curves of (002) and (101) plane reflection shows irradiation-induced broadening. Atomic force microscopy imagery revealed the formation of nanoclusters on the surface of the irradiated samples. X-ray photoelectron spectroscopy confirms that the surface features are composed of GaN. The effects of ion-beam-produced lattice defects on the surface, electrical, and optical properties of GaN were studied and possible mechanisms responsible for the formation of nanoclusters during irradiation have been discussed.