A novel organic hyperbranched copper phthalocyanine was synthesized for use as a hole injection nanolayer on ITO in organic light-emitting diodes (OLEDs). This material is soluble in organic solvents which allows for processing under anhydrous conditions, unlike water based conventional polymer hole injection layer materials such as poly(3,4-ethylenedioxythiophene)(PEDOT)/polystyrene sulfonate (PSS). The hyperbranched layer increased the luminous efficiency and brightness of single layer OLED devices, in addition to reducing current leakage which causes crosstalk in panel devices, compared to devices prepared from PEDOT/PSS. Therefore, this material is more suitable for OLED applications due to its processing and performance advantages over conventional commercial conducting polymer compositions.