Some particle size analyzers, such as the Par-Tec(R) 100 (Laser Sensor Technology, Redmond, WA, USA), measure the so-called cord length distribution (CLD) as the laser beam emitted from the sensor randomly crosses two edges of a particle (a cord length). The objectives of this study were to develop a model that can predict the response of the Par-Tec(R) 100 in measuring the CLD of a suspension for spherical and ellipsoidal particles and to infer the actual particle size distribution (PSD) using the measured CLD output. The model showed that the measured CLD is reasonably accurate for the spherical particles. However, this measurement progressively deteriorates as the shape of particles changes from spherical to ellipsoidal with large ratios of major to minor diameters. Experimental results obtained with spherical particles having a normal and a non-normal PSD indicated that the Par-Tec(R) 100 measurements deteriorate as the PSD deviates from a normal distribution. The information obtained from these experiments also showed that the model can reasonably predict the Par-Tec(R) response. Use of the inferred PSD rather than the measured CLD made a major improvement in estimating the actual PSD. Mean particle size analysis revealed that the Par-Tec(R) 100 volume-weighted mean particle size is closest to the unweighted mean particle size measured by sieve analysis.