Impact of acid-base conditions on defluoridation by induced crystallization

Linyu Deng; Ying Wang; Jianqi Zhou; Tinglin Huang; Xin Sun

Journal of Industrial and Engineering Chemistry, Vol.83, 35-45, March, 2020

DOI10.1016/j.jiec.2019.11.010 Export Citation

Impact of acid-base conditions on defluoridation by induced crystallization

Linyu Deng^{1, 2, †}, Ying Wang^{1, 2}, Jianqi Zhou^{1, 2}, Tinglin Huang^{1, 2}, and Xin Sun^{1, 2}

¹School of Environmental and Municipal Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China
²Key Laboratory of Northwest Water Resources, Environment and Ecology, Ministry of Education, Xi’an University of Architecture and Technology, Xi’an 710055, China

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Defluoridation by induced crystallization under extreme pH and bicarbonate/carbonate alkalinity of an aquatic environment was researched. At the conditions of initial pH 4-10 and alkalinity of less than 9.92 mM, the F- could be successfully removed by the induced crystallization of Ca5(PO4)3F on the PR surface within 1 h. With a prolonged time of 144 h, the F- could be also removed by the formation of Ca5(PO4)3F at initial pH 2 and alkalinity 9.92 mM. However, in extreme base aquatic environments, such as pH 12 or alkalinity 17.12 mM, the F- was partially removed by the induced crystallization of FCO3- apatite (Ca9.316Na0.36Mg0.144(PO4)4.8(CO3)1.2F2.48) and the F- could be completely removed by adjusting pH to a range of 4-10. Additionally, the safe disposal of spent crystal seed is successfully achieved as an extra benefit.

Keywords:Defluoridation;Induced crystallization;Initial pH;Initial alkalinity;Removal mechanisms

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[Referenced By]

[1] Ayoob S, Gupta AK, Crit. Rev. Environ. Sci. Technol., 36 (2006)

[2] WHO, Guidelines for Drinking-Water Quality, fourth ed., (2011) Geneva.

[3] Zhu C, Bai G, Liu X, Li Y, Water Res., 40 (2006)

[4] Reddy DV, Nagabhushanam P, Sukhija BS, Reddy AGS, Smedley PL, Chem. Geol., 269 (2010)

[5] Abu Jabal MS, Abustan I, Rozaimy MR, Al-Najar H, J. Afr. Earth Sci., 100 (2014)

[6] Rafique T, Naseem S, Usmani TH, Bashir E, Khan FA, Bhanger MI, J. Hazard. Mater., 171 (2009)

[7] Rafique T, Naseem S, Ozsvath D, Hussain R, Bhanger MI, Usmani TH, Sci. Total Environ., 530-531 (2015)

[8] Ayoob S, Gupta AK, Bhat VT, Crit. Rev. Environ. Sci. Technol., 38 (2008)

[9] Loganathan P, Vigneswaran S, Kandasamy J, Naidu R, J. Hazard. Mater., 248-249 (2013)

[10] Mumtaz N, Pandey G, Labhasetwar PK, Crit. Rev. Environ. Sci. Technol., 45 (2015)

[11] Palahouane B, Drouiche N, Aoudj S, Bensadok K, J. Ind. Eng. Chem., 22 (2015)

[12] Djouadi Belkada F, Kitous O, Drouiche N, Aoudj S, Bouchelaghem O, Abdi N, Grib H, Mameri N, Sep. Purif. Technol., 204 (2018)

[13] Ouslimane T, Aoudj S, Amara M, Drouiche N, Int. J. Environ. Res., 11 (2017)

[14] Macintire WH, Hammond JW, Ind. Eng. Chem., 30 (1938)

[15] Larsen MJ, Pearce EIF, Caries Res., 26 (1992)

[16] Pearce EIF, Larsen MJ, Caries Res., 27 (1993)

[17] Dahi E, WEDC, (1996).

[18] Deng L, Liu Y, Huang T, Sun T, Chem. Eng. J., 287 (2016)

[19] Zhang W, Ma W, Ji Y, Fan M, Oenema O, Zhang F, Nutr. Cycl. Agroecosyst., 80 (2008)

[20] Cooper J, Lombardi R, Boardman D, Carliell-Marquet C, Resour. Conserv. Recycl., 57 (2011)

[21] Malash GF, El-Khaiary MI, J. Colloid Interface Sci., 348 (2010)

[22] Ma QY, Logan TJ, Traina SJ, Environ. Sci. Technol., 29 (1995)

[23] Prasad M, Saxena S, Amritphale SS, Chandra N, Environ. Technol., 22 (2001)

[24] Kadouche S, Lounici H, Benaoumeur K, Drouiche N, Hadioui M, Sharrock P, J. Polym. Environ., 20 (2012)

[25] Lemlikchi W, Drouiche N, Belaicha N, Oubagha N, Baaziz B, Mecherri MO, J. Ind. Eng. Chem., 32 (2015)

[26] Featherstone JDB, Pearson S, LeGeros RZ, Caries Res., 18 (1984)

[27] Gustafsson JP, KTH Royal Institute of Technology Stockholm, Sweden, (2013).

[28] Elouear Z, Bouzid J, Boujelben N, Feki M, Jamoussi F, Montiel A, J. Hazard. Mater., 156 (2008)

[29] Yi H, Balan E, Gervais C, Segalen L, Fayon F, Roche D, Person A, Morin G, Guillaumet M, Blanchard M, Lazzeri M, Babonneau F, Am. Mineral., 98 (2013)

[30] Wei W, Cui J, Wei Z, Chemosphere, 105 (2014)

[31] Perrone J, Fourest B, Giffaut E, J. Colloid Interface Sci., 249 (2002)

[32] Correia LM, Campelo NDS, Novaes DS, Cavalcante CL, Cecilia JA, Rodriguez-Castellon E, Vieira RS, Chem. Eng. J., 269 (2015)

[33] Szilas C, Koch CB, Msolla MM, Borggaard OK, Geoderma, 147 (2008)

[34] Inskeep WP, Silvertooth JC, Geochim. Cosmochim. Acta, 52 (1988)

[35] Ge X, Ren C, Lu X, Li Z, Chen G, Wang K, Ren F, Wang Q, Wang M, An X, Qian B, Ceram. Int., 45 (2019)

[36] Ribeiro dos Santos V, Dezena Cabrelon M, de Sousa Triches E, Quinteiro E, J. Clean Prod., 240 (2019)

[37] Zhang Y, Zhang Z, Zhu M, Cheng F, Zhang D, Appl. Therm. Eng., 148 (2019)

[38] Hidalgo-Robatto BM, Aguilera-Correa JJ, Lopez-Alvarez M, Romera D, Esteban J, Gonzalez P, Serra J, Surf. Coat. Technol., 349 (2018)

[39] Nan N, Zhu Y, Han Y, Miner. Eng., 132 (2019)

[40] Han M, Zhang J, Hu Y, Han R, J. Chem. Eng. Data, 64 (2019)

[41] He Y, Zhang L, An X, Wan G, Zhu W, Luo Y, Sci. Total Environ., 688 (2019)

[42] Zhang YX, Jia Y, J. Colloid Interface Sci., 510 (2018)

[43] Telkapalliwar NG, Shivankar VM, Data in Brief, vol. 26 (2019).

[44] Jung KW, Hwang MJ, Jeong TU, Chau DM, Kim K, Ahn KH, J. Ind. Eng. Chem., 39 (2016)

[45] Mena VF, Betancor-Abreu A, Gonzalez S, Delgado S, Souto RM, Santana JJ, J. Environ. Manage., 246 (2019)