Polymer electrolyte membrane fuel cell (PEMFC) stacks suffer from the high cost and low volumetric energy of non-porous graphite bipolar plates. To resolve this problem, a bilayer coating consisting of Ni and Ni-Cr-P is deposited on AISI 1020 low-carbon steel using pulse electrodeposition. Ni/Ni-Cr-P-coated AISI 1020 is evaluated as a bipolar plate material for PEMFCs. Ni/Ni-Cr-P-coated substrates exhibit better corrosion resistance in both cathodic (air-purging) and anodic (H-2-purging) environment than the bare AISI 1020 substrate and lower interfacial contact resistance (ICR) than bare AISI 1020 and stainless steel. Further, it is expected to show better water management as the Ni/Ni-Cr-P coating is more hydrophobic than the bare substrate. Preliminary studies show that Ni/Ni-Cr-P-coated AISI 1020 plate can be a suitable candidate for replacing graphite as the bipolar plate of PEMFCs. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.