This paper presents high-fidelity flame structure measurements of premixed methane-air Bunsen flames subjected to extreme levels of turbulence. Specifically, 28 cases were studied with longitudinal integral length scales (L-x) as large as 43 mm, turbulence levels (u'/S-L) as high as 246, and turbulent Reynolds (Re-T,Re-0) and Karlovitz (Ka(T)) numbers up to 99,000 and 533, respectively. Two techniques were employed to measure the preheat and reaction layer thicknesses of these flames. One consisted of planar laser induced fluorescence (PLIF) imaging of CH radicals, while the other involved taking the product of simultaneously acquired PLIF images of formaldehyde (CH2O) and hydroxyl (OH) to produce "overlap-layers." The average preheat layer thicknesses are found to increase with increasing u'/St and with axial distance from the burner (x/D). In contrast, average reaction layer (i.e. CH- and overlap-layer) thicknesses did not increase appreciably even as u'/SL increased by a factor of 60. Furthermore, the reaction layer thicknesses (based on the CH images only) did not increase with increasing x/D. The reaction layers are also observed to remain continuous; that is, local extinction events are rarely observed. Although based on a sequence of combined CH-OH PLIF images acquired at a rate of 10 kHz, it is apparent that when instances of local extinction do occur they are the result of cool gas entrainment The results presented here, as well as those from 12 prior experimental and 9 numerical investigations, do not agree with the predicted Klimov-Williams boundary on the theoretical Borghi Diagram. Thus, a new Measured Regime Diagram is proposed wherein the Klimov-Williams criterion is replaced by a metric that relates the turbulent diffusivity (D-T = u'Lx) to the molecular diffusivity within the preheat layer (D* = S-L delta(F,L)). justification for this replacement is based on physical reasoning and the fact that the line defined by D-T/D* approximate to 180 accurately separates cases with thin flamelets from those with broadened preheat yet thin reaction layers (i.e. BP-TR flames). Additionally, the results suggest that the BP-TR regime extends well beyond what was previously theorized since neither broken nor broadened reaction layers were observed under conditions with Karlovitz numbers as high as 533, which is five times higher than the theoretical boundary. (C) 2017 The Combustion Institute. Published by Elsevier Inc. All rights reserved.