Bench scale tests were carried out to investigate the rheological properties of multi-sized particulate Bingham slurries at high solid concentrations ranging from 50% to 70% by weight. In addition, rheological data from Biswas et al. (2000) and Chandel et al. (2009, 2010) have also been considered. Based on these extensive amount of rheological data, an empirical model is proposed for viscosity as a function of solid volume fraction (?), maximum solid volume fraction (?(m)), median particle diameter (d(50)), and coefficient of uniformity (C-u) using optimization and nonlinear least-square curve-fitting technique. The proposed model shows good agreement with the experimental data considered in the present study and is found to be much better than the previously developed models in predicting the viscosity of multi-sized particulate Bingham slurries at high solid concentrations.