Phytochemical investigations on the above-ground parts of Lamium garganicum, subsp. laevigatum resulted in the isolation of 7 iridoid glucosides: shanzhiside methyl ester (1), barlerin (8-O-acetylshanzhiside methyl ester) (2), 6-O-syringl-8-O-acetylshanzhiside methyl ester (3), 6 beta-hydroxipolamide (4), lamalbide (5), dehydropenstemoside (6) mid sesamoside (7). The structure of the iridoids was elucidated by spectroscopic (UV, IR, 1D- ancl 2D-NNTR and ESI-MS) evidence.