Mechanical alloying was utilized to produce Cu80Fe20/CNT nano-composite powder. The effects of CNT addition on solid solubility of Fe in Cu, morphology, magnetic, and electrical properties of the products were evaluated using X-ray diffraction, field emission scanning electron microscopy, vibrating sample magnetometer, and four point probe technique, respectively. It was found that solid solubility of Fe in Cu increased to 20 wt.% in a sample milled for 15 h, but CNTs impeded the solid solubility extension in Cu80Fe20/CNT nano-composites. CNTs were distributed evenly in metal matrix after 15 h mechanical alloying and final products were agglomerates consisting of nano-particles. Analysis of magnetic hysteresis loops showed that the magnetic properties of nano-composite samples were altered as a function of CNT addition. Saturation magnetization and coercivity of composite samples increased with increasing CNT content probably due to the presence of non-dissolved Fe in nano-composites and exchange coupling phenomenon, respectively. Electrical resistivity of nano-composites also increased with increasing CNT concentration. (C) 2014 Elsevier B.V. All rights reserved.