International Journal of Heat and Mass Transfer, Vol.77, 17-21, 2014
Thermal properties of thin films studied by ultrafast laser spectroscopy: Theory and experiment
The one-dimensional non-homogeneous hyperbolic energy equation within a semi-infinite domain, applied to pump probe transient reflectance measurements for subpicosecond and picosecond laser pulses was studied. The result of this study is an analytical model in the form of a Volterra-type integral equation that describes the surface temperature response of the thin film induced by an ultra-short laser pulse and takes into account contributions of the transient heat flux and the volumetric heat source. The criterion based on dimensionless time xi(p) = t/2 tau (where tau is the relaxation time of phonons due to collisions) is introduced, in order to predict the temperature response caused by the surface heat flux and/or volumetric source. This analytical solution is validated by using experimental pump-probe transient reflectance measurements of thin gold with a time resolution of 50 fs. A good agreement between the experimental results and the theoretical model is found. (C) 2014 Elsevier Ltd. All rights reserved.