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Journal of Chemical Physics, Vol.106, No.5, 2045-2048, 1997
Coherent Control of Multiphoton Driven Processes - A Laser-Induced Catalyst
A well-known quantum interference phenomenon is combined with laser-induced collisional energy transfer to create a coherently controlled excitation involving two species. From one viewpoint the process involves a laser induced catalyst. An experimental demonstration is performed in mixtures of Xe and Kr gases.
Keywords:PUMPED STIMULATED EMISSIONS;3RD-HARMONIC GENERATION;MIXING INTERFERENCE;3-PHOTON RESONANCE;COOPERATIVE SHIFTS;IONIZATION;EXCITATION;SUPPRESSION;TRANSITIONS;COMPETITION