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Journal of Chemical Physics, Vol.104, No.4, 1173-1178, 1996
Optimal-Control of Population Transfer in an Optically Dense Medium
We apply the optimal control technique (OCT) to design an optical pulse pair that controls the population transfer in a medium of three-level atoms. The absorption and reshaping of the controlling pulses by the medium are taken into account. The efficiency of the population transfer is improved significantly compared with designs that do not incorporate pulse absorption and reshaping.
Keywords:ELECTROMAGNETICALLY INDUCED TRANSPARENCY;MULTILEVEL SYSTEMS;MOLECULAR-DYNAMICS;VIBRATIONAL LEVELS;PRODUCT FORMATION;PULSE;PHASE;FLUORESCENCE;SPECTROSCOPY;SELECTIVITY