화학공학소재연구정보센터
Journal of Canadian Petroleum Technology, Vol.48, No.8, 22-27, 2009
Onset of Convection in CO2 Sequestration in Deep Inclined Saline Aquifers
CO2 sequestration in deep geological formations has been suggested as an option to reduce greenhouse gas emissions. Saline aquifers are one of the most promising options for carbon dioxide storage. It has been shown that the dissolution of CO2 into brine causes the density of the mixture to increase. If the corresponding Rayleigh number of the porous medium is enough to initiate convection currents, the rate of dissolution will increase. Early time dissolution of CO2 in brine is mainly dominated by molecular diffusion, while late time dissolution is predominantly governed by a convective mixing mechanism. In this paper, linear stability analysis of density-driven miscible flow for carbon dioxide sequestration in deep inclined and homogeneous saline aquifers is presented. The effect of inclination and its influence on the pattern of convection cells has been investigated and the results are compared with the horizontal layer. The current analysis provides approximations for the initial wavelength of the convective instabilities and the onset of convection that helps in selecting suitable candidates for geological CO2 sequestration sites.